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2003 | 12 | 1 |

Tytuł artykułu

Transport and speciation of PAHs and PCBs in a river ecosystem

Warianty tytułu

Języki publikacji

EN

Abstrakty

EN
This paper presents the results of analysis of samples of river water and bottom sediments for PAH and PCB content using previously developed analytical procedures. Conclusions are drawn as to the form and main places of occurrence of the above analytes in the various elements of the river ecosystem (water phase, suspension, bottom sediments). The dependencies which were found between the PAH and PCB concentration in these three phases of the ecosystem suggest that: · PAHs are almost entirely adsorbed on the suspension and their transport in river water occurs mainly with the suspended matter. · PCBs are adsorbed to a lesser degree on the particles of suspended matter, which means that their transport in the river takes place both with the aqueous phase and with the suspended matter. · PAHs accumulate in bottom sediments to a much greater extent than PCBs.

Wydawca

-

Rocznik

Tom

12

Numer

1

Opis fizyczny

p.105-110,fig.,ref.

Twórcy

autor
  • Technical University of Gdansk, 11-12 Narutowicz Str., 80-952 Gdansk, Poland
autor
autor

Bibliografia

  • 1. SEŃCZUK W. Toksykologia. Wydawnictwo Lekarskie PZWL, Warszawa 1994.
  • 2. HOWTHORNE S. B., BJORKLUND E., BOWADT S., MATHIASSON L. Determining PCB sorption/desorption behaviour on sediments using selective supercritical fluid extraction 3. Sorption from water. Environ. Sci. Technol. 33, 3152, 1999.
  • 3. MITRA S., DICKHUT R. M., KUEHL S. A., KIMBROUGH K. L. Polycyclic aromatic hydrocarbons (PAH) source, sediment desorption patterns, and particle geochemistry as factors influencing PAH distribution coefficients in sediments of the Elizabeth River, VA , USA. Mar. Chem. 66, 113, 1999.
  • 4. LAW R. L., DAWES V. J., WOODHEAD R. J., MATTHIESSEN P. Polycyclic aromatic hydrocarbons (PAH) in seawater around England and Wales. Mar. Pol. Bull.34, 306, 1997.
  • 5. KUCKLICK J. R., BIDLEMAN T. F. Organic contaminants in Winyah Bay, South Carolina I: pesticides and polycyclic aromatic hydrocarbons in subsurface and microlayer water. Mar. Environ. Res. 37, 63, 1994.
  • 6. WOODHEAD R. J., LAW R. L., MATTHIESSEN P. Polycyclic aromatic hydrocarbons in surface sediments around England and Wales, and their possible biological significance. Mar. Pol. Bull. 38, 773, 1999.
  • 7. KOT A., NAMIEŚNIK J. The role of speciation in analytical chemistry. TrAC 19(2-3), 69, 2000
  • 8. WINKELS H. J., KROONENBERG S. B., LYCHAGIN M. Y., MARIN G., RUSAKOV G. V., KASIMOV N. S. Geochronology of priority pollutants in sedimentation zones on the Volga and Donube delta in comparison with the Rhine delta. Appl. Geochem.13, 581, 1998.
  • 9. READMAN J. W., MANTOURA R. F. C., RHEAD M. M. The physico-chemical speciation of polycyclic aromatic hydrocarbons (PAH) in aquatic systems. Fresenius J. Anal. Chem. 319, 126, 1984.
  • 10. VAN NOORT P. C. M., WONDERGEM E. The isolation of some polynuclear aromatic hydrocarbons from aqueous samples by means of reversed-phase concentrations columns. Anal. Chim. Acta 172 , 335, 1985.
  • 11. WOLSKA L., GALER K., GÓRECKI T., NAMIEŚNIK J. Surface water preparation procedure for chromatographic determination of polycyclic aromatic hydrocarbons and polychlorinated biphenyls. Talanta 50, 985, 1999.
  • 12. WOLSKA L., WIERGOWSKI M., GALER K., GÓRECKI T., NAMIEŚNIK J. Sample preparation for GC analysis of selected pesticides in surface water. Chemosphere 39, 1477, 1999.
  • 13.WOLSKA L. Miniaturized analytical procedure of determining polycyclic aromatic hydrocarbons and polychlorinated biphenyls in bottom sediments. J. Chromatogr.959, 173, 2002.
  • 14. KALAJZIC T., BIANCHI M., GAWLIK B., MUNTAN H., KETTRUP A. On the elimination of high-boiling impurities interfering with the analysis of polychlorinated biphenyls and organochlorinated pesticides in sediment samples. Ann. Chim. 89, 257, 1999.
  • 15.KOLB M., BOHM H. B., BAHADIR M. Analytical multimethod for the determination of low volatile organic pollutants in sediments and sewage sludges. Fresenius J. Anal. Chem.351, 286, 1995.
  • 16.LINDHARDT B., HOLST H., CHROTENSEN T. H. Comparison of soxhlet and shake extraction of PAH from coal far polluted soils sampled in the field. Intern. J. Environ. Anal. Chem.57, 9, 1994.
  • 17. NOTAR M., LESKOVSEK H. Determination of polycyclic aromatic hydrocarbons in marine sediments using a new ASESFE extraction technique. Fresenius J. Anal. Chem.366, 846, 2000.
  • 18. WOLSKA L., WARDENCKI W., WIERGOWSKI M., ZYGMUNT B., ZABIEGAŁA B., KONIECZKA P., POPRAWSKI L., BIERNAT J. F., NAMIEŚNIK J. Evaluation of pollution degree of the Odra river basin with organic compound after the 1997 summer flood - general comments. Acta Hydrochimica et Hydrobiologica 27, 343, 1999.
  • 19. HUALI Y., SHIFEN X., YONGRUI T., XIN J., JIANFANG F., SHUOKUI H., LIANSHENG W. The adsorption of PCBs to Yangtse river sediment. Toxicol. Environ. Chem. 76, 171, 2000.

Typ dokumentu

Bibliografia

Identyfikatory

Identyfikator YADDA

bwmeta1.element.agro-article-9cf0f964-6170-482c-ac73-df9c2d12aa4c
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