Decolorization of Reactive Red 239 using UV-C activated peroxydisulfate

• Autorzy: Kartal O.E.
• Języki publikacji: EN

Abstrakty

EN

Decolorization of Reactive Red 239 (RR239) using a sulfate radical (SO₄˙⁻ )-based advanced oxidation process was investigated in a batch photoreactor. SO₄˙⁻ was generated in situ through activation of peroxydisulfate under UV-C illumination. Effect of initial pH (3-9), initial dye concentration (20-50 mg dm⁻³), S₂O₈²⁻ dosage (0-3 mmol dm⁻³) and lamp power (0-16 W) were explored. It was found that initial pH of RR239 solution had no considerable effect on decolorization efficiency. Experimental results demonstrated that decolorization efficiency enhanced with increasing S₂O₈²⁻ dosage and lamp power and decreasing initial dye concentration. Quenching experiments were performed with alcohols to determine the dominant radical. Under the conditions tested in this study, 98% and 70% decolorization and aromatic degradation efficiencies were obtained within 120 min of irradiation time, respectively. Decolorization and aromatic degradation efficiencies of RR239 in PS/UV-C and PMS/UV-C systems were evaluated in terms of electrical energy consumption per order by figure of merit approach.

• Wydawca: -
• Czasopismo: Polish Journal of Environmental Studies
• Rocznik: 2019
• Tom: 28
• Numer: 5
• Opis fizyczny: p.3261-3267,fig.,ref.

Twórcy

autor

Kartal O.E.

• Department of Chemical Engineering, Inonu University, Malatya, Turkey

Bibliografia

• 1. YANG S., WANG P., YANG X., SHAN L., ZHANG W., SHAO X., NIU R. Degradation efficiencies of azo dye Acid Orange 7 by the interaction of heat, UV and anions with common oxidants: Persulfate, peroxymonosulfate and hydrogen peroxide. J. Hazard. Mater., 179, 552, 2012.
• 2. LAU T.M., CHU W., GRAHAM N.J.D. The aqueous degradation of butylated hydroxyanisole by UV/S2O8 2: Study of reaction mechanisms via dimerization and mineralization. Environ. Sci. Technol., 41, 613, 2007.
• 3. TAN C., GAO N., DENG Y., AN N., DENG J. Heat-activated persulfate oxidation of diuron in water. Chem. Eng. J., 203, 294, 2012.
• 4. CHEN J., ZHANG L., HUANG T., LI W., WANG, Y., WANG, Z. Decolorization of azo dye by peroxymonosulfate activated by carbon nanotube: Radical versus non-radical mechanism. J. Hazard. Mater., 320, 571, 2016.
• 5. ISMAIL L., FERRONATO C., FINE L., JABER F., CHOVELONA J.M. Elimination of sulfaclozine from water with SO₄⁻ radicals: Evaluation of different persulfate activation methods. Appl. Catal. B, 201, 573, 2017.
• 6. MAHDI-AHMED M., CHIRON S. Ciprofloxacin oxidation by UV-C activated peroxymonosulfate in wastewater. J. Hazard. Mater., 265, 41, 2014.
• 7. FRONTISTIS Z., HAPESHI E., FATTA-KASSINOS D., MANTZAVINOS D. Ultraviolet -activated persulfate oxidation of methyl orange: a comparison between artificial neural networks and factorial design for process modeling. Photochem. Photobiol. Sci., 14, 528, 2015.
• 8. SALARI D., NIAERI A., ABER S., RASOULIFARD M. H. The photooxidative destruction of C.I. Basic Yellow 2 using UV/S₂O₈²⁻ process in a rectangular continuous photoreactor. J. Hazard. Mater., 166, 61, 2009.
• 9. GHAUCH A., TUQAN A. M. Oxidation of bisoprolol in heated persulfate/H2O systems: Kinetics and products. Chem. Eng. J., 183, 162, 2012.
• 10. MORA V.C., ROSSO J.A., LE ROUX G.C., MARTIRE D.O., GONZALEZ M.C. Thermally activated peroxydisulfate in the presence of additives: A clean method for the degradation of pollutants. Chemosphere, 75, 1405, 2009.
• 11. ANTONIOU M.G., DE LA CRUZ A.A., DIONYSIOU D.D. Degradation of microcystin-LR using sulfate radicals generated through photolysis, thermolysis and e−transfer mechanisms. App. Catal. B, 96, 290, 2010.
• 12. NIPSITAKIS G.P., DIONYSIOU D.D. Radical generation by the interaction of transition metals with common oxidants. Environ. Sci. Technol., 38, 3705, 2004.
• 13. HU P., LONG M. Cobalt-catalyzed sulfate radical-based advanced oxidation: A review on heterogeneous catalysts and applications. App.Catal. B, 181, 103, 2016.
• 14. NASSERI S., MAHVI A.H., SEYEDSALEHI M., YAGHMAEIAN K., NABIZADEH R., ALIMOHAMMADI M., SAFARI G.H. Degradation kinetics of tetracycline in aqueous solutions using peroxydisulfate activated by ultrasound irradiation: Effect of radical scavenger and water matrix. J. Mol. Liq., 241, 704, 2017.
• 15. ULLAH I., ALİ S., HANİF M.A., ZİA. M.A. Photocatalytic activity of Al₂O₃‧Fe₂O₃ synthesized by ultrasonic-assisted mechanical stirring. Pol. J. Environ. Stud., 26, 2777, 2017.
• 16. ASGHAR A., RAMAN A.A.A., DAUD W.M.A.W. Advanced oxidation processes for in-situ production of hydrogen peroxide/hydroxyl radical for textile wastewater treatment: a review. J. Clean. Prod. 87, 826, 2015.
• 17. FANG G.-D., DIONYSIOU D. D., ZHOU D.-M., WANG Y., ZHU X.- D., FAN J.- X., CANG L., WANG Y.- J. Transformation of polychlorinated biphenyls by persulfate at ambient temperature. Chemosphere, 90, 1573, 2013.
• 18. SAIEN J., SOLEYMANI A.R., SUN J.H. Parametric optimization of individual and hybridized AOPs of Fe²⁺/H₂O₂ and UV/S₂O₈²⁻ for rapid dye destruction in aqueous media. Desalination, 279, 298, 2011.
• 19. LIANG C., WANG Z.- S., BRUELL C.J. Influence of pH on persulfate oxidation of TCE at ambient temperatures. Chemosphere, 66, 106, 2007.
• 20. CHEN X., XUE Z., YAO Y., WANG W., ZHU F., HONG C. Oxidation degradation of Rhodamine B in aqueous by UV/S₂O₈²⁻ treatment system. Int. J. Photoenergy, 2012, Article ID 754691, 2012.
• 21. OLMEZ-HANCI T., ARSLAN-ALATON İ. Comparison of sulfate and hydroxyl radical based advanced oxidation of phenol. Chem. Eng. J. 224, 10, 2013.
• 22. RASTOGI A., AL-ABED S.R., DIONYSIOU D.D. Sulfate radical-based ferrous-peroxymonosulfate oxidative system for PCBs degradation in aqueous and sediment systems. App. Catal. B, 85, 171, 2009.
• 23. DING Y., ZHU L., WANG N., TANG H. Sulfate radicals induced degradation of tetrabromobisphenol A with nanoscaled magnetic CuFe₂O₄ as a heterogeneous catalyst of peroxymonosulfate. App. Catal. B, 129, 153, 2013.
• 24. ANIPSITAKIIS G.P., DIONYSIOU D.D., GONZALEZ M.A. Cobalt-mediated activation of peroxymonosulfate and sulfate radical attack on phenolic compounds. Implications of chloride ions. Environ. Sci. Technol., 40, 1000, 2006.
• 25. SAIEN J., MORADI V., SOLEYMANI A.-R. Investigation of a jet mixing photo-reactor device for rapid dye discoloration and aromatic degradation via UV/H₂O₂ process. Chem. Eng. J., 183, 135, 2012.
• 26. KHATAEE A.R., PONS M.N., ZAHRAA O. Photocatalytic degradation of three azo dyes using immobilized TiO₂ nanoparticles on glass plates activated by UV light irradiation: Influence of dye molecular structure. J. Hazard. Mater., 168, 451, 2009.
• 27. WANG P., YANG S., SHAN L., NIU R., SHAO X. Involvements of chloride ion in decolorization of Acid Orange 7 by activated peroxydisulfate or peroxymonosulfate oxidation .J. Environ. Sci., 23, 1799, 2011.
• 28. CHEN J., GAO N., LU X., MENG M., GU Z., JIANG C., WANG Q. Degradation of 2,4-dichlorophenol from aqueous using UV activated persulfate: kinetic and toxicity investigation. RSC Adv., 6, 100056, 2016.
• 29. KHATAEE A.R. Application of central composite design for the optimization of photodestructionof a textile dye using UV/S₂O₈²⁻ process. Pol. J. Chem.Tech., 11, 38, 2009.
• 30. SHARMA J., MISHRA I.M., KUMAR V., Degradation and mineralization of Bisphenol A (BPA) in aqueous solution using advanced oxidation processes: UV/H₂O₂ and UV/S₂O₈²⁻ oxidation systems. J. Environ. Manage., 156, 266, 2015.

Identyfikatory

DOI

10.15244/pjoes/94049