Polycyclic aromatic hydrocarbons in the particles emitted from the diesel and gasoline engines

• Autorzy: Szewczynska M. , Dabrowska J. , Pyrzynska K.
• Języki publikacji: EN

Abstrakty

EN

Polycyclic aromatic hydrocarbons (PAHs) are contaminants widespread in the environment and vehicular emissions have long been recognized as the most important anthropogenic sources of PAHs in urban air Polycyclic aromatic hydrocarbons (PAHs) emitted in the exhaust gases of diesel and petrol engines using different fuels were quantified. Size fractionated chemical analysis of particles in vehicle emissions were carried out by sampling with an electrical low pressure multi-stage impactor ELPI. The mean concentrations of total PAHs adsorbed onto the particulate matter in the rage of 0.03-0.25 μm emitted from the exhaust gases were 48.3, 128.2 and 83.0 ng·m⁻³, respectively from three kinds of diesel fuels. Results indicated that PAHs present in the last two fraction (0.17-0.25 μm) have the highest contribution in the total content of these compounds. In the collected fractions of particulate matter emitted in gasoline engine exhaust 12 compounds were identified in the 0.25 µm fraction and 9 PAHs in the 0.17 µm fraction.

• Wydawca: -
• Czasopismo: Polish Journal of Environmental Studies
• Rocznik: 2017
• Tom: 26
• Numer: 2
• Opis fizyczny: P.801-807,fig.,ref.

Twórcy

autor

Szewczynska M.

• Centralny Instytut Ochrony Pracy- PIB, Czerniakowska 16, 00-701 Warszawa, Poland

autor

Dabrowska J.

• University of Warsaw, Chemistry Department, Pasteura 1, 02-093 Warsaw, Poland

autor

Pyrzynska K.

• University of Warsaw, Chemistry Department, Pasteura 1, 02-093 Warsaw, Poland

Bibliografia

• 1. VU T.V., DELGADO-SABORIT J.M., HARRISON R.M., Review: Particle number size distributions from seven major sources and implications for source apportionment studies. Atmos. Environ. 122, 114, 2015.
• 2. TOBISZEWSKI M., NAMIEŚNIK J. PAH diagnostics ratios for the identification of pollution emission sources. Environ. Pollut. 162, 110, 2012.
• 3. FERNANDEZ-GONZALEZ V., CONCHA-GRANA E., MUNIATEGA-LORENZO S., LOPEZ-MAHIA P., PRADA-RODRIGEZ D., Solid-phase microextraction-gas chromatographic - tandem mass spectrometric analysis of polycyclic aromatic hydrocarbons. Towards the European Union water directive 2006/0129 EC, J. Chromatogr. A 1176, 48, 2007.
• 4. BETHA R., BALASUBRAMANIAN R., Emissions of particulate-bound elements from stationary diesel engine: Characterization and risk assessment, Atmos. Environ. 45, 5273, 2011.
• 5. VILLENEUVE P.J., PARENT M.E, SAHNI V., JOHNSON K.C. Occupational exposure to diesel and gasoline missions and lung cancer in Canadian men, Environ. Res. 111, 727, 2011
• 6. HIEN T.T., THANH L., KAMEDA T., TAKENAKA N., BANDOW H., Distribution characteristics of polycyclic aromatic hydrocarbons with particle size in urban aerosols at roadside in Ho Chi Minh, Vietnam. Atmos. Environ. 41, 1575, 2007
• 7. HE C., GE Y., MA C., TAN J., LIU Z., WANG C., YU L.X., DING, Y., Emission characteristics of a heavy-duty diesel engine at simulated high altitudes, Sci. Tot. Environ. 409, 3138, 2011.
• 8. CHIANG H.L., LAI Y.M., CHANG S.Y., Pollutant constituents of exhaust emitted from light-duty diesel vehicles, Atmos. Environ. 47, 399, 2012.
• 9. KAM W., LIACOS J.W., SCHAUER J.J., DELFINO R.J., SIOUTAS, C., Size-segregated composition of particulate matter (PM) in major roadways and surface streets. Atmos. Environ. 55, 90, 2012.
• 10. SZEWCZYŃSKA M., POŚNIAK M., DOBRZYŃSKA E., PYRZYNSKA K., BARANIECKA J. Polycyclic aromatic hydrocarbons distribution in fine and ultrafine particles emitted from diesel engine to the air. Pol. J. Environ. Stud. 22, 553, 2013.
• 11. SZEWCZYŃSKA M., POŚNIAK M., DOBRZYŃSKA E., Study on individual PAHs content in ultrafine particles from solid fractions of diesel and biodiesel exhaust fumes, e-Journal of Chemistry, 2013, Article ID 528471. http://dx.doi.org/10.1155/2013/528471
• 12. KARJALAIMEN P., OIRRJOLA L., HEIKKILÄ J., LÄHDE T., TZAAMKIZOS T., NTZIACHRISTOS L., KOSKINEN J., RŐNKŐ T., Exhaust particles of modern gasoline vehicles: A laboratory and on-road study. Atmos. Environ. 97, 262, 2014.
• 13. ASHRAFUL A.M., MASJUKI H.H., KALAM M.A., Particulate matter, carbon emissions and elemental compositionjs from a diesel engine exhaust fuelled with diesel-biodiesel blends. Atmos. Environ. 100, 463, 2015.
• 14. WORLD HEALTH ORGANIZATION. International Agency for Research on Cancer, Press release No. 213. 2012.
• 15. RAVINDRA K., SOKHI R., VAN GRIEKEN R., Atmospheric polycyclic aromatic hydrocarbons: source attribution, emission factors and regulation. Atmos. Environ. 42, 2895, 2008.
• 16. MATHISSEN M., SCHEER V., VOGT R., BENTER T., Investigation on the potential generation of ultrafine particles from the tire-road interface. Atmos. Environ. 45, 6172, 2011.
• 17. LIACOS J.W., KAM W., DELFINO R.J., SCHAUER J.J., SIOUTAS C., Characterization of organic, metal and trace element PM₂.₅ species and derivation of freeway-based emission rates in Los Angeles. CA. Sci. Total Environ. 435, 159, 2012.
• 18. KHAIRY M.A., LOHMANN R., Source apportionment and risk assessment of polycyclic aromatic hydrocarbons in the atmospheric environment of Alexandria, Egypt. Chemosphere 91, 895, 2013.
• 19. LIU Y., GAO Y., ZHANG C., WANG S., MA L., ZHAO J., LOHMANN, R. Particulate matter, gaseous and particle polycyclic aromatic hydrocarbons (PAHs) in an urban traffic tunnel of China: Emission from on-road vehicles and gas-particle partitioning. Chemosphere 134, 52, 2015.
• 20. MARJAMÄKI M., LEMMETTY M., KESKINEN J., ELPI response and data reduction. I: Response functions. Aeros. Sci. Technol. 39, 575, 2005.
• 21. BARANIECKA J., PYRZYNSKA K., SZEWCZYŃSKA M., POŚNIAK M., DOBRZYŃSKA E., Emission of polycyclic aromatic hydrocarbons from selected processes in steel works. J. Hazard. Mater. 183, 111, 2010.
• 22. MOTELAY-MASSEI A., HARNER T., SHOEIB M., DIAMOND M., STERN G., ROSENBERG, B., Using passive air samplers to assess urbane rural trends for persistent organic pollutants and polycyclic aromatic hydrocarbons. 2. Seasonal trends for PAHs, PCBs, and organochlorine pesticides. Environ. Sci. Technol. 39, 5763, 2005.
• 23. CALLEN M.S., LOPEZ J.M., MASTRAL A.M., Apportionment of the airborne PM10 in Spain. Episodes of potential negative impact for human health. J. Environ. Monit. 14, 1211, 2012.
• 24. CRISTALE J., SILVA F.S., ZOCOLO G.J., MARCHI M.R., Influence of sugarcane burning on indoor/outdoor PAH air pollution in Brazil. Environ. Pollut. 169, 210, 2012.
• 25. AYDIN Y.M., KARA M., DUMANOGLU Y., ODABASI M., ELBIR T. Source apportionment of polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) in ambient air of an industrial region in Turkey. Atmos. Environ. 97, 271, 2014.
• 26. TIAN Y.Z., LI W.H., SHI G.L., FENG Y.C.,WANG Y.Q. Relationships between PAHs and PCBs, and quantitative source apportionment of PAHs toxicity in sediments from Fenhe reservoir and watershed. J. Hazard Mater. 248, 89, 2013.
• 27. GUO H., LEE S.C., HO K.F., WANG X.M., ZOU S.C., Particle-associated polycyclic aromatic hydrocarbons in urban air of Hong Kong. Atmos. Environ. 37, 5307, 2003.
• 28. GUNAWARDENA J., EGODAWATTA P., AYOKO G.A., GOONETILLEKE A., Role of traffic in atmospheric accumulation of heavy metals and polycyclic aromatic hydrocarbons. Atmos. Environ. 54, 502, 2012.
• 29. WHO Guidelines for Indoor Air Quality: Selected Pollutants, World Health Organization, Copenhagen 2010.

Identyfikatory

DOI

10.15244/pjoes/64914