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2018 | 27 | 1 |

Tytuł artykułu

Advanced treatment of paper-making wastewater using catalytic ozonation with waste rice straw-derived activated carbon-supported manganese oxides as a novel and efficient catalyst

Autorzy

Warianty tytułu

Języki publikacji

EN

Abstrakty

EN
Waste rice straw was converted into activated carbon-supported manganese oxides (MnOx/RSAC) that were first used as a catalyst to improve the performance of ozonation of real paper-making wastewater. The results indicated that catalytic ozonation with the prepared catalyst exhibited a highly efficient performance in advanced treatment of paper-making wastewater, and the corresponding color and COD removal efficiencies were 58.5 and 77.5%, respectively. And the treated wastewater was more biodegradable and less toxic than that in ozone alone. Based on significant inhibition of the radical scavenger and fluorescence test in the catalytic ozonation process, we deduced that the enhancement of catalytic activity was responsible for MnOx/RSAC catalyzing ozone to generate more hydroxyl radicals and the possible reaction pathway was proposed. Thus, MnOx/RSAC catalyzing ozonation could serve as a stable, efficient, and economical process with a potential engineering application for treated refractory wastewater, and the results offered new insights for sustainable use of waste rice straw.

Słowa kluczowe

Wydawca

-

Rocznik

Tom

27

Numer

1

Opis fizyczny

p.451-457,fig.,ref.

Twórcy

autor
  • Key Laboratory of Recycling and Eco-treatment of Waste Biomass of Zhejiang Province, Zhejiang University of Science and Technology, Hangzhou, China
autor
  • Key Laboratory of Recycling and Eco-treatment of Waste Biomass of Zhejiang Province, Zhejiang University of Science and Technology, Hangzhou, China
autor
  • Key Laboratory of Recycling and Eco-treatment of Waste Biomass of Zhejiang Province, Zhejiang University of Science and Technology, Hangzhou, China

Bibliografia

  • 1. ASHRAFI O., YERUSHALMI L., HAGHIGHAT F., Wastewater treatment in the pulp-and-paper industry: A review of treatment processes and the associated greenhouse gas emission. J. Environ. Manage. 158, 146, 2015.
  • 2. HERMOSILLA D., MERAYO N., GASCO A., BLANCO Á. The application of advanced oxidation technologies to the treatment of effluents from the pulp and paper industry: a review. Environ. Sci. Pollut. Res. 22, 168, 2015.
  • 3. BUYUKKAMACI N., KOKEN E. Economic evaluation of alternative wastewater treatment plant options for pulp and paper industry. Science of the Total Environment. 408, 6070, 2010.
  • 4. LUCAS M.S., PERES J.A., AMOR C., MALDONADO M.I., MALATO S. Tertiary treatment of pulp mill wastewater by solar photo-Fenton. J. Hazard. Mater, 225-226, 173, 2012.
  • 5. RODRIGUES A.C., BOROSKI M., SHIMADA N.S., GARCIA J.C., NOZAKI J. Treatment of paper pulp and paper mill wastewater by coagulation-flocculation followed by heterogeneous photocatalysis. J. Photoch. Photobio. A. 194, 1, 2008.
  • 6. ASGHAR M.N., KHAN S., MUSHTAQ H. Management of treated pulp and paper mill effl uent to achieve zero discharge. J. Environ. Manage. 88, 1285, 2008.
  • 7. FARIA P.C.C., ORFAO J.J.M., PEREIRA M.F.R. Activated carbon and ceria catalysts applied to the catalytic ozonation of dyes and textile effluents. Applied Catalysis B: Environmental. 88, 341, 2009.
  • 8. ZHUANG H.F., HAN H.J., HOU B.L., JIA S.Y., ZHAO Q. Heterogeneous catalytic ozonation of biologically pretreated Lurgi coal gasifi cation wastewater using sewage sludge based activated carbon supported manganese and ferric oxides as catalysts. Bioresour Technol. 166, 178, 2014.
  • 9. KASPRZYK-HORDERN B., ZIOLEK M., NAWROCKI J. Catalytic ozonation and methods of enhancing molecular ozone reactions in water treatment. Appl. Catal. B-Environ. 46, 639, 2003.
  • 10. WANG H., QUAN B.X., AN X.Q., YANG Y., TIAN C. Advanced decomposition of coking wastewater in relation to total organic carbon using an electrochemical system. Pol. J. Environ. Stud. 26, 941, 2017.
  • 11. CHU Y.Y., ZHU M.G., LIU C. Electrochemical treatment of biotreated landfill leachate using a porous carbon nanotubecontaining cathode: Performance, toxicity reduction, and biodegradability enhancement. Environ. Eng. Sci. 32, 445, 2015.
  • 12. HUANG Y., CUI C., ZHANG D. Heterogeneous catalytic ozonation of dibutyl phthalate in aqueous solution in the presence of iron-loaded activated carbon. Chemosphere. 119, 295, 2015.
  • 13. ZANG A.D., GRATHWOHL P. Enhanced immobilization of polycyclic aromatic hydrocarbons in contaminated soil using forest wood-derived biochar and activated carbon under saturated conditions, and the importance of biochar particle size. Pol. J. Environ. Stud. 25, 427, 2016.
  • 14. SUI M.H., XING S.C., SHENG L., HUANG S.H., GUO H.G. Heterogeneous catalytic ozonation of ciprofloxacin in water with carbon nanotube supported manganese oxides as catalyst. J. Hazard. Mater, 227-228, 227, 2012.
  • 15. TORRELLAS S.A., LOVERA R.G., ESCALONA N., SEPULVEDA C., SORELO J.L., GARCIA J. Chemicalactivated carbons from peach stones for the adsorption of emerging contaminants in aqueous solutions. Chem. Eng. J. 279, 788, 2015.
  • 16. APHA, Standard Methods for the Examination of Water and Wastewater, 18thed. 1992, Washington, DC: American Public Health Association.
  • 17. HE S.M., LI J., XU J., MO L.H. Enhanced removal of COD and color in paper-making wastewater by ozonation catalyzed by Fe supported on activated carbon. BioResources. 11, 8396, 2016.
  • 18. ESPLUGAS S., CINTRERAS S., OLLIS D. Engineering aspects of the integration of chemical and biological oxidation: simple mechanistic models for the oxidation treatment. J. Envir. Eng. 130, 967, 2004.
  • 19. ZHANG H.F., HAN H.J., SHAN S.D. Treatment of British Gas/Lurgi coal gasification wastewater using a novel integration of heterogeneous Fenton oxidation on coal fly ash/sewage sludge carbon composite and anaerobic biological process. Fuel. 178, 155, 2016.
  • 20. IKHLAQ A., BROWN D.R., Kasprzyk-Hordern B. Mechanisms of catalytic ozonation on alumina and zeolites in water: Formation of hydroxyl radicals. Appl. Catal. B: Environ. 123-124, 94, 2012.

Typ dokumentu

Bibliografia

Identyfikatory

Identyfikator YADDA

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